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Professor Turnbull served as a visiting lecturer at the University of Canterbury, Christchurch, NZ in 1995, and as a visiting professor at the Universitat de Barcelona, Spain in 2001-2002.
Our research lies in the preparation of new materials and is focused in two areas.
Molecular Magnetism
Over the last two decades, a new field of research has emerged called molecular magnetism. The guiding principle is to use our understanding of structure, bonding and geometry to control the bulk magnetic properties of a material at the molecular level. This is highly interdisciplinary work and involves teams of collaborating organic and inorganic chemists, theoreticians and condensed matter physicists (our group works in collaboration with that of Prof. Christopher Landee in the Physics Dept. as well as several groups around the world, including Spain, Germany, Great Britain and New Zealand).Low-dimensional Antiferromagnets
The copper oxide-based high temperature superconductors have introduced a new era to the field of conducting materials, but the mechanism of their superconductivity is still not well understood. One theory suggests that the mechanism of the electrical superconductivity is related to the mechanism of magnetic super-exchange in these compounds. We are working to prepare structurally related complexes which have more moderate ordering tempertures as models for these systems and others where the magnetic interactions are not principally propagated in 3-dimensions. Of special interests are those materials where the magnetic interactions are not strictly one- or two-dimensional in nature, but whose topology may be described as inter-dimensional, such as ladders, honeycombs and rectangles. We have recently succeeded in preparing a large family of the best examples of magnetic ladders known (at right) and experiments are in progress to determine their properties and whether doping the systems will generate superconducting materials as predicted by theory.Degrees
- Ph.D. in Organic Chemistry, Brandeis University, 1987
- M.S. in Inorganic Chemistry, University of New Hampshire, 1984
- B.S. in Chemistry, University of New Hampshire, 1978
Affiliated Department(s)
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Scholarly and Creative Works
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Diaqua-bis(2,2’-bipyridine)dinitratooxalatodicopper(II)
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2021
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The Synthesis, Structure, and Magnetic Properties of a Family of Mn(II) Compounds with Substituted 2-aminopyridinium Ions
Polyhedron
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2021
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A new lead-free 1D hybrid copper perovskite with structural, thermal, vibrational, optic and magnetic characterizations
Journal of Materials Chemistry C
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2021
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Design, synthesis and physico-chemical studies of a novel Co(II)/Co(III) mixed-valence complex: An experimental and DFT approach
Journal of Molecular Structure
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2021
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Vol. 1237
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Synthesis, structure and magnetic properties of catena-diaqua-bis(pyridine-N-oxide)(μ-pyrazine)copper(II) perchlorate and the monomeric structure tetrakis(pyridine-N-oxide)copper(II) perchlorate
Journal of Coordination Chemistry
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2021
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Vol. 74
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Two New Canted Antiferromagnetic Systems: Magnetic, Theoretical, and Crystallographic Studies on trans-Bis(2-Iodopyridine)dihalocopper(II)
Dalton Transactions
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2021
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Vol. 50
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“Synthesis, structure and magnetic properties of catena-diaqua-bis(pyridine-N-oxide)(μ-pyrazine)copper(II) perchlorate and the monomeric structure tetrakis(pyridine-N-oxide)copper(II) perchlorate”
Journal of Coordination Chemistry
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2021
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Vol. 74
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“The Synthesis, Structure, and Magnetic Properties of Nickel (II) 6-Coordinate Species with Several Substituted Aniline Ligands”
Polyhedron
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2021
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Vol. 200
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Polymorphism in the metal-organic hybrid (PhCH2NEt3)2[CoBr4]: Synthesis, crystal structures and physico-chemical characterizations
Inorganica Chimica Acta
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2021
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Vol. 514
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catena(2,2’-bipyridine)oxalatocopper(II)
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2020
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catena-bis(2,3-dimethylpyrazine)trichloridotricopper(I)
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2020
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Diaquabis(pyrazine-2-carboxylato)copper(II)
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2020
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Bis(2-amino-3-hydroxypyridinium) tetrachloridocuprate(II)
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2020
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“Well-isolated pyrazine-bridged copper(II) chains: Synthesis and magneto-structural analysis”
Journal of Coordination Chemistry
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2020
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Vol. 73
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“Pyrazine-bridged Cu(II) chains: diaquabis(n-methyl-2-pyridone)copper(II) perchlorate complexes”
Dalton Transactions
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2020
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Vol. 49
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Extremely well-isolated 2D spin-1/2 antiferromagnetic Heisenberg layers with small exchange coupling in the molecular-based magnet CuPOF
Physics Reviews B
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2020
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Vol. 102
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Synthesis, Crystal structure and magnetic properties of Bis(3-amino-2-chloropyridine)-dibromidocopper(II)
European Chemical Bulletin
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2020
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Vol. 9
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Structural Correlations in Low-Dimensional Cu(II)-based Molecular Magnetic Materials
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Multiple locations (see description)
2019-2020
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2020
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Magnetic order and disorder in a quasi-two-dimensional quantum Heisenberg antiferromagnet with randomized exchange
Phys. Rev. B
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2020
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Vol. 102
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Assessing Cu2L2X4 dimeric moieties as ferromagnetic building blocks in double halide-bridged polymers (X = Cl-, Br- and L = benzamide). An experimental and computational study
Polyhedron
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2020
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Vol. 185
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Cobalt halide complexes of 2-, 3- and 4-methoxyaniline: syntheses, structures and magnetic behavior
Polyhedron
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2020
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Vol. 187
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Structure and Magnetic Properties of a Serendipitously Synthesized Copper(II) Complex: [Cu(3-Br-2-pyone)6](ClO4)2
Trans. Metal Chem
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2020
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Vol. 45
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catena-bis(2,3-dimethylpyrazine)trichloridotricopper(I)
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2020
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Diaquabis(pyrazine-2-carboxylato)copper(II)
2020
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2020
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Bis(2-amino-3-hydroxypyridinium) tetrachloridocuprate(II)
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2020
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Copper(II) halide salts with 1-(4’-pyridinium)-pyridinium
Inorganics
2020
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2020
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Vol. 8
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Issue #18
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A new mixed halide 2d hybrid perovskite: structural, thermal, optic and magnetic properties
Polyhedron
2020
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2020
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Issue #175
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Syntheses, structures and properties of copper(II) and cobalt(II) complexes with 5(3)-amino-2-chloro-3(5)-methylpyridine isomer cations
Inorg. Chim. Acta
2020
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2020
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Issue #500
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Solvothermal synthesis, structural characterization, DFT and magnetic studies of a Cu(II)-metallamacrocycle
J. Mol. Struct.
2020
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2020
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Issue #1201
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Low-Dimensional Cu(II)-based Molecular Magnetic Materials; Benefits of hydroxypyridine/pyridone ligands
MAGnetism in North America
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St. Simons Island, GA
February 21-24
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2020
Sponsored by MAGnetism in North America
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Synthesis and EPR Studies of Pyrazine-Bridged Copper (II) Complexes (oral and poster, presented by Emma Kirkman-Davis)
MAGNA 2020 (conference on MAGnetism in North America)
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St. Simons Island, GA
February 21-24
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2020
Sponsored by MAGnetism in North America
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Magnetism and structure of 6- and 4-coordinate nickel complexes with substituted aniline ligands (oral and poster, presented by Katherine Meehan)
MAGNA 2020 (conference on MAGnetism in North America)
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St. Simons Island, GA
February 21-24
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2020
Sponsored by MAGnetism in North America
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Revisiting the Role of Hydrogen Bonding in the Strong Dimer Superexchange of a 2D Copper(II) Halide Honeycomb-Like Lattice: Structural and Magnetic Study
Inorg Chem
2020///
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2020
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Vol. 59
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Tetrakis(4-methylpyridine)copper(II) perchlorate
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2019
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Tetrakis(4-methylpyridine)copper(II) tetrafluoroborate
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2019
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Tetrakis(4-nitropyridine-N-oxide)copper(II) perchlorate
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2019
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Bis(2-amino-6-methylpyridinium) tetrachlorocuprate(II)
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2019
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Catena 2-amino-6-methylpyridinium trichlorocuprate (II)
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2019
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Bis (4-methylpyridinium) tetrabromidocuprate(II)
2019
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2019
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Bispyridinium tetrabromidocuprate(II)
2019
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2019
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Synthesis and structural and magnetic characterization of an Iron(III) pyrophosphate complex with 1,10’-phenanthroline
Inorganica Chimica Acta
2019
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2019
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Diversity of Coordination Modes in a Flexible Ditopic Ligand Containing 2-pyridyl, Carbonyl and Hydrazone Functionalities: Mononuclear and Dinuclear Cobalt(III) Complexes, and Tetranuclear Copper(II) and Nickel(II) Cluster
Magnetochemistry
2019
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2019
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Vol. 5
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Issue #39
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Synthesis, structure and magnetic properties of a binuclear Co(II)-pyrophosphate complex, [Co2(phenanthroline-dione)4(P2O7)]”
Polyhedron
2019
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2019
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Issue #170
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Halide-bi-bridged polymers of amide substituted pyridines: Polymorphism, structures and magnetism
CrystEngComm
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2019
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Vol. 21
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Issue #1910-27
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What? Wait a minute? The liberal arts include science? Yes!
Higher Education Consultants Association (HECA)
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Crowne Plaza Hotel, Warwick, RI
June 17-21
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2019
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Well-isolated 2D-antiferromagnetic copper(II) complexes
42nd Northeast Regional Meeting of the American Chemical Society
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Saratoga Springs, NY
June 23-26
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2019
Sponsored by American Chemical Society
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Antiferromagnetic exchange of n-methyl-2-pyridone substituted copper(II) pyrazine linear chains (presented by F. Witkos)
42nd Northeast Regional Meeting of the American Chemical Society
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Saratoga Springs, NY
June 23-26
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2019
Sponsored by American Chemical Society
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Synthesis and characterization of a hole doped 2D-QHAF: (quinolinium)2CuxZn1-xBr4●2H2O (presented by J.C. Monroe)
42nd Northeast Regional Meeting of the American Chemical Society,
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Saratoga Springs, NY
June 23-26
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2019
Sponsored by American Chemical Society
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Systematic synthesis and study of magnetism of copper-based adamantoid structures (presented by S. Fowles)
42nd Northeast Regional Meeting of the American Chemical Society
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Saratoga Springs, NY
June 23-26
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2019
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Structure, coordination and magneto-structural correlations of nickel (II) with substituted aniline ligands (presented by K. Meehan)
42nd Northeast Regional Meeting of the American Chemical Society
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Saratoga Springs, NY
June 23-26
●
2019
Sponsored by American Chemical Society
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EPR studies of pyrazine-bridged copper (II) chains with pyridone ligands (presented by E. Kirkman-Davis)
42nd Northeast Regional Meeting of the American Chemical Society
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Saratoga Springs, NY
June 23-26
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2019
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Cobalt and zinc halide complexes of 4-chloro and 4-methylaniline: Syntheses, structures and magnetic behavior.
Polyhedron
2019///
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2019
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Vol. 168
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Pyridine-based complexes of copper(II) chloride and bromide: ligand conformation effects on crystal structure. Synthesis, structure and magnetic behavior of Cu(2-Cl-3-X'py)2X2 [X, X' = Cl, Br].
J. Coord. Chem.
2019///
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2019
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Vol. 72
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Issue #11
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Halide-bridged Cu(pyrazine)2 perchlorate layers: Structure and magnetism.
Polyhedron
2019///
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2019
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Vol. 171
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Unusual coordination behavior by a hydroxypyridine/pyridone ligand: Synthesis and structure of [ (2-bromo-4-hydroxypyridine)2(2-bromo-1(H)-4-pyridone)2copper(II)] perchlorate • 2(2-bromo-4-hydroxypyridine) • 2(2-bromo-1(H)-4-pyridone)”
J. Coord. Chem.
2019
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2019
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Vol. 72
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Issue #19-21
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Effects of deuteration on the structure and magnetic properties of (quinolinium)2 tetrabromidocuprate(II) dihydrate
J. Coord. Chem.
2019///
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2019
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Vol. 72
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Issue #22-24
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Eur. Chem. Bull.
2019
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2019
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Vol. 8
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Issue #5
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Crystal structure of 2-bromo-4-hydroxypyridine: hydrogen and halogen bonding.
Eur. Chem. Bull.
2019
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2019
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Vol. 8
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Issue #6
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Eur. Chem. Bull.
2019
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2019
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Vol. 8
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Issue #8
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Synthesis, structure, and magnetic properties of a family of copper(II) complexes and salts of isoquinoline: (Isoquinoline)nCu(X)2 [X = Cl, Br] and (isoquinolinium)2CuX4(H2O)n [X =Cl, Br; n = 0,1].
Polyhedron
2018///
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2018
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Vol. 147
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Copper(II) halide complexes of aminopyridines: Syntheses, structures and magnetic properties of [(5CAP)2CuX2] and [(5BAP)nCuX2] (X = Cl, Br).
J. Coord. Chem.
2018///
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2018
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Vol. 71
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Issue #16-18
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Transition metal salts of quinoline: synthesis, structure and magnetic behavior of (QuinH)2[MX4]·2H2O [Quin = quinoline; M = Mn, Co, Cu, Zn], (QuinH)2[MnBr2(H2O)2](Br)2 and (QuinH)[Cu(Quin)Br3].
J. Coord. Chem.
2018///
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2018
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Vol. 71
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Issue #20
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2-Chloro-3-fluoropyridine copper(II) complexes and the effect of structural changes on magnetic behavior.
J. Coord. Chem.
2018///
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2018
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Vol. 71
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Issue #21
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Bistability in Organic Magnetic Materials: A Comparative Study of the Key Differences between Hysteretic and Non-hysteretic Spin Transitions in Dithiazolyl Radicals
Chemistry
2017///
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2017
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Vol. 23
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Issue #14
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Field induced spontaneous quasiparticle decay and renormalization of quasiparticle dispersion in a quantum antiferromagnet
Nat Commun
2017///
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2017
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Vol. 8
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Quantum criticality in the spin-1/2 Heisenberg chain system copper pyrazine dinitrate
Sci Adv
2017///
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2017
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Vol. 3
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Issue #12
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Copper(II) halide salts and complexes of 4-amino-2-fluoropyridine: synthesis, structure and magnetic properties.
J. Coord. Chem.
2017///
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2017
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Vol. 70
●
Issue #5
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Ferromagnetic Exchange in Bichloride Bridged Cu(II) Chains: Magnetostructural Correlations between Ordered and Disordered Systems.
Inorg. Chem.
2017///
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2017
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Vol. 56
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Issue #9
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Transition metal salts of 2-amino-3,5-dihalopyridine - dimers: syntheses, structures and magnetic properties of (3,5-diCAPH)2Cu2Br6 and (3,5-diBAPH)2Cu2X6.
J. Coord. Chem.
2017///
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2017
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Vol. 70
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Issue #23
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A unique copper(ii)-assisted transformation of acetylacetone dioxime in acetone that leads to one-dimensional, quinoxaline-bridged coordination polymers
Dalton Trans
2016///
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2016
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Vol. 46
●
Issue #1
-
Eur. Chem. Bull.
2016///
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2016
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Vol. 5
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Issue #2
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Mechanochemical synthesis of [L nCuX 2] (L = 3-cyanopyridine, 2-amino-3-cyanopyridine, 2-amino-5-cyanopyridine; n = 1, 2; X = Cl, Br) via drop-solvent grinding.
Mechanochemical synthesis of [L nCuX 2] (L = 3-cyanopyridine, 2-amino-3-cyanopyridine, 2-amino-5-cyanopyridine; n = 1, 2; X = Cl, Br) via drop-solvent grinding.2016///
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2016
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Structural, magnetic susceptibility, and EPR results for a family of weakly interacting copper(II) halide compounds with 1,4'-bipyridinium.
Structural, magnetic susceptibility, and EPR results for a family of weakly interacting copper(II) halide compounds with 1,4'-bipyridinium.2016///
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2016
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Mechanochemical synthesis of copper(II) halide complexes: Synthesis, structure and magnetic properties of 2-amino-5-bromo- and 2-amino-5-chloropyridine complexes.
Mechanochemical synthesis of copper(II) halide complexes: Synthesis, structure and magnetic properties of 2-amino-5-bromo- and 2-amino-5-chloropyridine complexes.2016///
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2016
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Transition metal complexes of 2-amino-3,5-dihalopyridines: Synthesis, structures and magnetic properties of (3,5-diCAP) 2Cu 2X 6 and (3,5-diBAP) 2Cu 2X 6.
Transition metal complexes of 2-amino-3,5-dihalopyridines: Synthesis, structures and magnetic properties of (3,5-diCAP) 2Cu 2X 6 and (3,5-diBAP) 2Cu 2X 6.2016///
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2016
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Synthesis, structure, and magnetic behavior of nickel (II) and cobalt (II) halide complexes of isoquinoline.
Synthesis, structure, and magnetic behavior of nickel (II) and cobalt (II) halide complexes of isoquinoline.2016///
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2016
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Field-induced quantum criticality and universal temperature dependence of the magnetization of a spin-1/2 heisenberg chain
Phys Rev Lett
2015///
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2015
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Vol. 114
●
Issue #3
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Synthesis, structure and magnetic properties of copper(II) complexes of 2-amino-5-trifluoromethylpyridine (5-TFMAP): (5-TFMAP)2CuX2 (X = Cl or Br), (5-TFMAP)3CuBr2 and [(5-TFMAP)2CuBr2](5-TFMAPH)Br.
Polyhedron
2015///
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2015
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Vol. 89
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Investigation of a well isolated 2-dimensional quantum Heisenberg antiferromagnetic model; EPR and SQUID studies of (quinolinium)2Cu1-xZnxX4 2H2O.
Investigation of a well isolated 2-dimensional quantum Heisenberg antiferromagnetic model; EPR and SQUID studies of (quinolinium)2Cu1-xZnxX4 2H2O.2015///
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2015
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The effect of 2-pyridone substitutions on the magnetic exchange of pyrazine in 2-pyridone/pyrazine linear chain complexes of copper (II) perchlorate.
The effect of 2-pyridone substitutions on the magnetic exchange of pyrazine in 2-pyridone/pyrazine linear chain complexes of copper (II) perchlorate.2015///
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2015
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The mechanochemical synthesis of 2-amino-5-substitutedpyridine copper (II) halide complexes and their magnetic properties.
The mechanochemical synthesis of 2-amino-5-substitutedpyridine copper (II) halide complexes and their magnetic properties.2015///
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2015
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Synthesis, structure, and magnetic behavior of a family of copper(II) halide/isoquinoline salts and complexes.
Synthesis, structure, and magnetic behavior of a family of copper(II) halide/isoquinoline salts and complexes.2015///
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2015
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Copper(II) halide salts and complexes of 4-amino-2-fluoropyridine: Synthesis, structure and magnetic properties.
Copper(II) halide salts and complexes of 4-amino-2-fluoropyridine: Synthesis, structure and magnetic properties.2015///
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2015
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Unusual redox reactions in the synthesis of copper coordination compounds: The synthesis of bis(5-NAP)CuCl2 and multiple polymorphs of bis(5-NAPH)CuCl4.
Unusual redox reactions in the synthesis of copper coordination compounds: The synthesis of bis(5-NAP)CuCl2 and multiple polymorphs of bis(5-NAPH)CuCl4.2015///
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2015
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Review. A gentle introduction to magnetism. Units, fields, theory, and experiment.
J. Coord. Chem.
2014///
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2014
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Vol. 67
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Issue #3
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Copper(II) complexes of 2-amino-5-chloro-3-fluoropyridine: syntheses and magnetic properties of (3,5-FCAP)2CuX2 and (3,5-FCAPH)2CuX4.
J. Coord. Chem.
2014///
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2014
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Vol. 67
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Issue #23-24
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Eur. Chem. Bull.
2014///
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2014
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Vol. 3
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Issue #2
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S=1/2 One-Dimensional Random-Exchange Ferromagnetic Zigzag Ladder, Which Exhibits Competing Interactions in a Critical Regime.
Chem. - Eur. J.
2014///
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2014
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Vol. 20
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Issue #27
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Phenazin-5-ium hydrogen sulfate monohydrate
Acta Crystallogr Sect E Struct Rep Online
2013///
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2013
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Vol. 69
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Issue #Pt 4
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Synthesis, structure, and magnetism of two tetrahalocuprate salts: (5-TFAPH)2CuX4 (5-TFAP = 2-amino-5-trifluoromethylpyridine, X = Cl, Br).
Polyhedron
2013///
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2013
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Vol. 52
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Recent Developments in Low-Dimensional Copper(II) Molecular Magnets.
Eur. J. Inorg. Chem.
2013///
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2013
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Vol. 2013
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Issue #13
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Effects of halogen and hydrogen bonding on defect disorder. The ladder that wasn't there.
CrystEngComm
2013///
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2013
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Vol. 15
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Issue #21
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Crystallographic and magnetic studies of the 2-pyridone/copper halide system.
Polyhedron
2013///
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2013
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Vol. 64
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Synthesis, structure, and magnetic behavior of [Cu2(pyrazine)3(CH3O)2](ClO4)2.
Eur. Chem. Bull.
2013///
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2013
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Vol. 2
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Issue #11
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Aqua(azido)[N-(pyridin-2-ylcarbonyl)pyridine-2-carboxamido-κ3N,N',N'']copper(II).
Acta Crystallogr., Sect. E: Struct. Rep. Online
2013///
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2013
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Vol. 69
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Issue #11
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3,4-Dihydroxy-1,6-bis(4-methoxyphenyl)hexa-2,4-diene-1,6-dione, its 4-methylphenyl analogue, and a potassium salt of 2-hydroxy-4-(4-methoxyphenyl)-4-oxobut-2-enoic acid.
Acta Crystallogr., Sect. C: Cryst. Struct. Commun.
2013///
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2013
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Vol. 69
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Issue #11
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Copper(II) catalyzed oxidation of 2-aminomethyl-pyridine: synthesis and structure of [(N,N-bis(2-pyridinecarbonyl)imidato-κN)(pyridine-2-carbonylamide-κO)copper(II)] nitrate dihydrate.
Eur. Chem. Bull.
2013///
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2013
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Vol. 2
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Issue #12
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Catena-bis(aqua(3-oxy-2-pyridono)copper(II))μ-pyrazine diperchlorate: a perchlorate-bridged magnetic ladder.
J. Coord. Chem.
2012///
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2012
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Vol. 65
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Issue #17
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Synthesis, structure, and magnetic behavior of a pyrazine-bridged Cu(II)/Au(CN)2 complex.
J. Coord. Chem.
2011///
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2011
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Vol. 64
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Issue #1
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Transition metal halide salts of 8-methylquinolinium: Synthesis and structures of (8-methylquinolinium)2MX4·nH2O (M = Cu, Co, Zn; X = Cl, Br; n = 0, 1).
Inorg. Chim. Acta
2011///
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2011
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Vol. 368
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Issue #1
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Two-dimensional spin-(1)/(2) rectangular Heisenberg antiferromagnets: Simulation and experiment.
Phys. Rev. B: Condens. Matter Mater. Phys.
2011///
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2011
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Vol. 84
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Issue #10
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Random exchange in the spin ladder Cu(quinoxaline)X2 (X = Cl, Br).
Polyhedron
2011///
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2011
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Vol. 30
●
Issue #18
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Two-dimensional spin-(1)/(2) rectangular Heisenberg antiferromagnets: Simulation and experiment [Erratum to document cited in CA156:683008].
Phys. Rev. B: Condens. Matter Mater. Phys.
2011///
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2011
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Vol. 84
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Issue #22
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Magnetism of extended arrays in inorganic solids.
Magnetism of extended arrays in inorganic solids.2011///
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2011
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Crystal structure and magnetism of a well isolated 2D-quantum Heisenberg antiferromagnet, (Quinolinium)(2)CuBr(4).2H(2)O, and its anhydrous form
Inorg Chem
2010///
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2010
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Vol. 49
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Issue #2
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Synthesis, structure, and magnetic properties of bis(monosubstituted-pyrazine)dihalocopper(II).
Dalton Trans.
2010///
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2010
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Vol. 39
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Issue #11
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Co(II) halide complexes with 2-amino-3-methyl-pyridinium and 2-amino-5-methyl-pyridinium: synthesis, crystal structures, and magnetic properties.
J. Coord. Chem.
2010///
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2010
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Vol. 63
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Issue #13
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An extremely well isolated 2D-antiferromagnetic layer.
Inorg. Chem. Commun.
2010///
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2010
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Vol. 13
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Issue #12
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Structure and Magnetism of Copper Pyrazine Chains Separated by Dicyanoaurate.
Structure and Magnetism of Copper Pyrazine Chains Separated by Dicyanoaurate.2010///
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2010
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Covalently-bridged spin ladders: Variable exchange through diazine ligands.
Covalently-bridged spin ladders: Variable exchange through diazine ligands.2010///
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2010
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Synthesis, crystal structure and effect of 2-pyridone substitution on pyrazine mediated magnetic exchange of 2-pyridone/pyrazine linear chains of copper (II) perchlorate.
Synthesis, crystal structure and effect of 2-pyridone substitution on pyrazine mediated magnetic exchange of 2-pyridone/pyrazine linear chains of copper (II) perchlorate.2010///
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2010
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Pyrazine-bridged 2-D QHAFs: Highly isolated systems.
Pyrazine-bridged 2-D QHAFs: Highly isolated systems.2010///
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2010
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Synthesis and magnetic interactions in low-dimensional copper halides coordination polymers.
Synthesis and magnetic interactions in low-dimensional copper halides coordination polymers.2010///
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2010
-
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Awards & Grants
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PCI Synthesis Summer Research Fellowship
PCI Synthesis
Jun. 1, 2021 - Aug. 31, 2021
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